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High efficiency of metal-complex catalysts on the basis of immobilized on silica ionic liquids in the radical processes has been established. They have shown their worth as stable initiators of the reactions that are of importance to the environmental protection. Namely they are: the oxidation of mercaptans in nonpolar medium, that is of oil purification current interest, and the radical-chain interaction of CCl4 with alkanes, that leads to the functionalization of hydrocarbons and utilization of waste perchlomethane.