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The interaction of micelles generated in aqueous solutions of polyisobutylene-block-poly(methacrylic acid) diblock copolymers with poly(N-ethyl-4-vinylpyridinium bromide) was demonstrated to result in the formation of water-soluble micellar interpolyelectrolyte complexes representing novel macromolecular architectures of "core-shell-corona" ("onion"-like) structure.