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New multifunctional material based on ferromagnetic barium ferrite particles, ferroelectric PZT particles and elastic polymer was prepared in the work. The research of magnetic and electrical properties of the elastomers revealed opposite magnetodeformation and magnetoelectric effects. The experimental data confirmed the mutual influence of FM and FE particles in elastic matrix. New ferromagnetic-ferroelectric-polymer composite is promising material both for the research in multifunctional materials area and for applications in sensor and memory devices.